HomeMy WebLinkAboutNC0000175_Cyanide Standards Letter_19990817UnImin
Quartz Operation
P. O. Box 588
Bakersville Hwy.
Spruce Pine, NC 28777
(828) 765 -4283
Fax: (828) 765 -0912
August 12, 1999
Mr. David A. Goodrich
NPDES Unit Supervisor
NCDEHNR
P. O. Box 29535
Raleigh, NC 27626 -0535
Dear Mr. Goodrich:
_ WA�Ek DUA
This is to acknowledge receipt of the information on site specific standards for
cyanide as developed for the Alcoa facility. That information is being reviewed by the
three feldspar producing companies for applicability to the fluoride standard.
Sincerely,
av i 4—
Charles F. Stover
Regional General Manager
CC: Dennis Buchanan – K T Feldspar
Tom Freeman – The Feldspar Corporation
Cyanide Options for Alcoa
I- Site - specific standard.
A. Eligibility per G.S. 143- 2143(b)
1. Natural background conditions in the stream segment preclude the attainment of the
applicable water quality standards; or
2. Irretrievable and uncontrollable man - induced conditions preclude the attainment of the
applicable water quality standards; or
3. Application of effluent limitations for existing sources established or proposed
pursuant to G.S. 143 -215.1 which are more restrictive than those effluent standards and
limitations determined or promulgated by the US EPA pursuant to section 301 of the
Federal Water Pollution Control Act (CWA) in order to achieve and maintain applicable
water quality standards would result in adverse social and economic impact,
disproportionate to the benefits to the public health, safety or welfare as a result of
maintaining the standards; wd
4. There exists no reasonable relationship between the cost to the petitioner of achieving
the effluent limitations necessary to comply with applicable water quality standards to the
benefits, including the incremental benefits to the receiving waters, to be obtained from
the application of the said effluent limitations.
B. Required Documentation
1. Compliance with all other NPDES permit requirements
2. Evaluation of sources and source reduction plan
3. Audit to assure proper function and management of facility
4. Pollution prevention plan tit verification of implementation
5. Cost analysis of all available treatments
6. Understanding that the discharger will receive a lower permit limit, if, the site- specific
standard is less than current state standard.
C. Steps for Approval
1. Approval of site - specific study results by Water Quality Staff
2. Compliance with G.S. 143 -2143 and section 301 of the CWA. These regulations state
that the new effluent limit nay not endanger human health and may not be less than either
�.; . the current effluent guidelines for the discharger or the highest level of treatment which
can reasonable be attained without economic hardship.
3. Compliance with state antidegradation policy (15A NCAC 2B .0201) must be
determined prior to issuance or reissuance of any site - specific effluent limits. Existing
uses must be protected by the site - specific water quality standard.
4. Approval by EMC through public hearing process.
D. Study Plan
1. If one of the G.S. 143-2143(b) requirements is judged by the EMC to be satisfactorily
met, then the facility will provide Water Quality staff with a study plan demonstrating
how sufficient data will be collected to develop a site- specific standard.
2. The discharger's permit limits will be based on the site - specific standard, even if the
site - specific standard is lower than the applicable water quality standard.
3. Study plans must be approved by Water Quality Staff
E. Methodologies
1. Recalculation Procedure - per 2nd Edition of EPA's Water Quality Standards
Handbook.
2. Indicator Species Procedure - per 2nd Edition of EPA's Water Quality Standards
Handbook.
3. Resident Species Procedure - per 2nd Edition of EPA's Water Quality Standards
Handbook.
II- We could change in standard to free cyanide. Could be added to Triennial Review and be final in
summer of 1996. In the meantime, they could conduct biological studies to determine aquatic life effects
and methodology studies to decrease variability in free cyanide determination. Would require WET testing
of particulate and free cyanide to document protection of aquatic life. Fate of lead- cyanide compounds
instream?
Ohio has recalculated free cyanide standard for warm and cold water. warm water is 12 ug/1 and cold water
is 52 ug/1. Water Quality Standards Coordinator is not aware of any problems with standard or discharges
has been on the books since 1989. He is checking with permitting folks to see number of dischargers and if
they are aware of any problems.
May 18,1995
OUTLINE FOR ALCOA CYANIDE FATE & TRANSPORT STUDY
ASSUMPTIONS
- facility is seeldng site specific standard based on recalculation and limited as Cyanide Amenable
to Chlorination (CATC)
- discharge 013 is legitimate effluent channel and not waters of state
- discharge of 013 does not circumvent requirements of solid/hazardous waste
-CN WQ standard is protective of primary human contact (Class B)
- facility has demonstrated compliance with all other effluent parameters including whole effluent
toxicity
Treatment/Discharge Considerations
- discussion of discharge alternatives
- discussion of treatment alternatives
- discussion of diffuser alternatives and potential for discharge to existing diffuser
- clarification that discharge permitting -for 013 will not circumvent intentions of groundwater or
solid/hazardous waste regulations applicable to site.
Characterization of CN discharge concentrations and factors that influence levels
-flow variables including spring flow and rainfall and relationship of each to total flow.
- concentration relative to rainfall
- consideration of load issues relative to the above
Cyanide Sampling
-water samples of 013 cove including samples immediately within swimming area.
- sediment samples within 013 cove including samples immediately within swimming area.
-water samples surrounding 012 discharge
- sediment samples surrounding 012 discharge
Characterization of species of cyanide and fate
- Analysis of total cyanide vs. CATC and characterization of the presence and percentage of
cyanide as iron cyanides.
- Evaluation of fate of cyanide including time and light dependent dissociation.
(in situ vs. in vitro ?)
- Evaluation of light penetration at both discharges and influence on potential for
photodecomposition
- characterization of known interferences to CN analysis
Biological sampling
- demonstration that benthic macroinvertebrate populations are not impacted by either discharge
through comparison with reference sites.
-If existing benthic populations are insufj`iceint for evaluation of impact AND sediment cyanide
samples report positive values, demonstrate lack of sediment toxicity through sediment toxicity
analyses using Chironomus tentans or Hyallella azteca per EP
-for use of site specific standard - demonstration that species removed from original criteria are
not present in the receiving waters and that all EPA recalculation guidance is followed.
Approval of Study PIan by DEM
Evaluation of study results by Div. Health Services and County Health Dept. relative to swimming
contact issues
Conclusions that should be reached for site specific limit and standard to continue
-Study plan has been approved by DEM, facility has completed study plan, and results are
acceptable to DENS.
- discharge to surface waters is the most ecologically /cost viable alternative
LA/DMR Page 1 June 9, 1995
OUTLLNE FOR ALCOA CYANIDE FATE & TRANSPORT STUDY
- alternatives analysis demonstrates that all treatment options are too costly.
- diffusion at 013 or via 012 is not cost effective
- discharge and permitting of this leachate from a hazardous waste site is appropriate
- consideration of the lake as the receiving water vs. the streamflow from the spring is
appropriate.
- studies should show that levels of CN are not toxic and not likely to become toxic in the water
column before dilution has reached the WQ std for totaL
- concentrations in the sediment anre not accumulating to the point where dissociation from the
sediment would exceed toxic levels
- benthic macroinvert. communities are not being affected by either discharge
-human health is not jeopardized by discharge of free or total cyanide levels (particularly
fromexposure at the.swimming beach).
-for site specific standard through recalculation- demonstration that species removed from
criteria, for purposes-of recalculation, are not present.
LA/DMR Page 2 June 9,1995
CYANIDE INFO SHEET
North Carolina Surface Water Quality Standard Development for Cyanide
• Adopted in 1979
• Based on EPA 'Red Book "1 chronic value of 5.0 ug/l for free cyanide.
• Implemented as total cyanide due to lack of reliable analytical method for measuring
free cyanide in wastewater.
• Federal Cyanide Standard Development
- 1976 'Red Book" chronic value of 5.0 ug/1 -
- 1980 Criteria document2 chronic value of 3.5 ug/l .
- 1985 Criteria document3 chronic value of 5.2 ug/l
• Reviewed in 1986. No changes made based on use of questionable acute /chronic ratio
in 1980 and fact that there is very little difference between the 5.0 and 5.2 ug/L
• 1994 EPA recommended the "Cyanide Amenable to Chlorine" (CATC) method for
analysis of free cyanide in DRINKING WATER4. It should be noted that drinking
water is not going to have the same interference potential as leachate, stormwater
runoff and spring water.- Standard- Methods states that CATC is useful for natural_
and groundwaters and clean metal finishing, heat treating & sanitary effluents. Some
unidentified organic chemicals may oxidize or form breakdown products during
chlorination, giving higher results for CATC than before chlorination. CATC based
on rapid dissociation of cyanide and eomplexing with chloramine -T.
Chemistry6
• "Cyanide" refers to all the CN groups that can be determined as the cyanide ion, CN-
• Ratio of CN- to HCN depends on pH & dissociation constant for HCN (pKa - 9.2)
• HCN is most toxic form.
• In natural waters HCN predominates.
• Decreased pH = increased HCN = increased toxicity.
• Simple metal cyanides vary in solubility but are highly soluble in complexes with alkali
(sodium, potassium, ammonium) cyanides.
• Synergistic toxic effects occur when zinc & copper ions combine with cyanide. .
• Iron cyanides do not dissociate easily. However, iron cyanides dissociation through
photodecomposition. 10 mg/l iron cyanide =1 mg/l HCN in strong sunlight, distilled
water.
• Dilution, mixing, clarity of the receiving waters & quantity of HCN released must be
assessed
• ASTM recommends that total cyanide determination be used to ensure good waste
treatment practices and states that there is a mistaken belief that the enumerated
cyanide compounds are not "toxic ". "The fact is that the toxicity is only of a lesser
magnitude." 1
Options for Cyanide Standard Implementation for Alcoa
• Status Quo - Implement current standard as total cyanide.
• Site - specific criteria development, see NC Site - specific criteria development guidance.
Requires special study and rule- making. Discharge cannot be toxic at IWC.
DMR/5/23/95
1 Quality Criteria for Water July 1976. US EPA.
2 Ambient Water Quality Criteria for Water. EPA 440/5 - 80-037.
3 Ambient Water Quality Criteria for Water. EPA 440/5 -84 -028.
4 57 FR 31776; July 17, 1992
5 Standard Methods for the Examination of Water and Wastewater, 17th Edition. 1989. APHA, AWWA
& WPCF.
6 1992 Annual Book of ASTM Standards Section 11, page 94 & Differential Toxicity of Fors of
Cyanide, 1990, prepared for The Aluminum Association.
7 Ibid. page 97.